Over 17.1% or 18.2% Efficiency of Layer-by-Layer All-Polymer Solar Cells via Incorporating Efficient Pt Complexes as Energy Donor Additive

Layer-by-layer (LbL) all-polymer solar cells (APSCs) are constructed with or without the incorporation of a Pt complex F-Pt as an energy donor additive in the acceptor layer. The power conversion efficiency (PCE) of LbL APSCs can be enhanced from 15.86% to 17.14% through introducing 0.2 wt % F-Pt in...

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Published inACS materials letters Vol. 6; no. 7; pp. 2964 - 2973
Main Authors Zhang, Lu, Zhang, Miao, Ni, Yuheng, Xu, Wenjing, Zhou, Hang, Ke, Shengyi, Tian, Hongyue, Jeong, Sang Young, Woo, Han Young, Wong, Wai-Yeung, Ma, Xiaoling, Zhang, Fujun
Format Journal Article
LanguageEnglish
Published American Chemical Society 01.07.2024
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Abstract Layer-by-layer (LbL) all-polymer solar cells (APSCs) are constructed with or without the incorporation of a Pt complex F-Pt as an energy donor additive in the acceptor layer. The power conversion efficiency (PCE) of LbL APSCs can be enhanced from 15.86% to 17.14% through introducing 0.2 wt % F-Pt in the PY-IT layer, originating from the efficient energy transfer from F-Pt to PM6 and PY-IT. The efficient energy transfer from F-Pt to PM6 and PY-IT can be well confirmed from the spectral overlapping between photoluminescence (PL) spectra of F-Pt and absorption spectra of PM6 and PY-IT, as well as the prolonged PL lifetime of PM6 and PY-IT according to the transient time-resolved PL spectra of blend and LbL films. The universality of the F-Pt incorporation strategy can be further confirmed from PBQx-TCl/PY-DT based LbL APSCs, and PCE can be increased from 17.57% to 18.29% by incorporating F-Pt into the PY-DT layer.
AbstractList Layer-by-layer (LbL) all-polymer solar cells (APSCs) are constructed with or without the incorporation of a Pt complex F-Pt as an energy donor additive in the acceptor layer. The power conversion efficiency (PCE) of LbL APSCs can be enhanced from 15.86% to 17.14% through introducing 0.2 wt % F-Pt in the PY-IT layer, originating from the efficient energy transfer from F-Pt to PM6 and PY-IT. The efficient energy transfer from F-Pt to PM6 and PY-IT can be well confirmed from the spectral overlapping between photoluminescence (PL) spectra of F-Pt and absorption spectra of PM6 and PY-IT, as well as the prolonged PL lifetime of PM6 and PY-IT according to the transient time-resolved PL spectra of blend and LbL films. The universality of the F-Pt incorporation strategy can be further confirmed from PBQx-TCl/PY-DT based LbL APSCs, and PCE can be increased from 17.57% to 18.29% by incorporating F-Pt into the PY-DT layer.
Author Zhang, Miao
Tian, Hongyue
Zhang, Lu
Jeong, Sang Young
Ma, Xiaoling
Woo, Han Young
Xu, Wenjing
Ke, Shengyi
Zhang, Fujun
Ni, Yuheng
Zhou, Hang
Wong, Wai-Yeung
AuthorAffiliation Organic Optoelectronic Materials Laboratory, Department of Chemistry, College of Science
Department of Applied Biology and Chemical Technology
Key Laboratory of Luminescence and Optical Information, Ministry of Education
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Snippet Layer-by-layer (LbL) all-polymer solar cells (APSCs) are constructed with or without the incorporation of a Pt complex F-Pt as an energy donor additive in the...
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Title Over 17.1% or 18.2% Efficiency of Layer-by-Layer All-Polymer Solar Cells via Incorporating Efficient Pt Complexes as Energy Donor Additive
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