Single-Atom Electrocatalysts for Lithium Sulfur Batteries: Progress, Opportunities, and Challenges

Lithium sulfur (Li–S) battery is considered as one of the most promising energy storage devices, because of its low cost, high energy density, and environmental friendliness. However, the practical applications of Li–S batteries have been hindered by a low utilization efficiency of sulfur arising fr...

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Published inACS materials letters Vol. 2; no. 11; pp. 1450 - 1463
Main Authors Wang, Feifei, Li, Jing, Zhao, Juan, Yang, Yixiao, Su, Chenliang, Zhong, Yu Lin, Yang, Quan-Hong, Lu, Jiong
Format Journal Article
LanguageEnglish
Published American Chemical Society 02.11.2020
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Abstract Lithium sulfur (Li–S) battery is considered as one of the most promising energy storage devices, because of its low cost, high energy density, and environmental friendliness. However, the practical applications of Li–S batteries have been hindered by a low utilization efficiency of sulfur arising from complicated chemical conversion of polysulfides and the corrosion of Li metal electrode during charge/discharge processes. Single atom catalysts (SACs) consisting of atomically-dispersed metal sites have been recently exploited as high-performance electrocatalytic materials in various energy storage devices, including Li–S batteries, because of their unique catalytic properties and maximized atom efficiency. In this mini-review, we first describe the major roadblocks and opportunities for the development of commercial Li–S batteries. Following that, we will highlight the specific roles of SAC materials, which are used as cathodes, separators, interlayers, electrolytes, and anodes in Li–S batteries. The detailed catalytic conversion mechanism of polysulfides and nucleation process of Li ions over single-atom active sites are also discussed. Finally, we highlight major challenges to be addressed in this field and provide our perspectives in the rational design and synthesis of superior SACs to accelerate their application in Li–S batteries.
AbstractList Lithium sulfur (Li–S) battery is considered as one of the most promising energy storage devices, because of its low cost, high energy density, and environmental friendliness. However, the practical applications of Li–S batteries have been hindered by a low utilization efficiency of sulfur arising from complicated chemical conversion of polysulfides and the corrosion of Li metal electrode during charge/discharge processes. Single atom catalysts (SACs) consisting of atomically-dispersed metal sites have been recently exploited as high-performance electrocatalytic materials in various energy storage devices, including Li–S batteries, because of their unique catalytic properties and maximized atom efficiency. In this mini-review, we first describe the major roadblocks and opportunities for the development of commercial Li–S batteries. Following that, we will highlight the specific roles of SAC materials, which are used as cathodes, separators, interlayers, electrolytes, and anodes in Li–S batteries. The detailed catalytic conversion mechanism of polysulfides and nucleation process of Li ions over single-atom active sites are also discussed. Finally, we highlight major challenges to be addressed in this field and provide our perspectives in the rational design and synthesis of superior SACs to accelerate their application in Li–S batteries.
Author Su, Chenliang
Yang, Quan-Hong
Lu, Jiong
Zhao, Juan
Wang, Feifei
Li, Jing
Zhong, Yu Lin
Yang, Yixiao
AuthorAffiliation Department of Chemistry
Nanoyang Group, State Key Laboratory of Chemical Engineering, School of Chemical Engineering and Technology
SZU-NUS Collaborative Center, International Collaborative Laboratory of 2D Materials for Optoelectronic Science & Technology of Ministry of Education, Engineering Technology Research Center for 2D Materials Information Functional Devices and Systems of Guangdong Province, Institute of Microscale Optoelectronics
Centre for Clean Environment and Energy, School of Environment and Science
Centre for Advanced 2D Materials and Graphene Research Centre
Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University
AuthorAffiliation_xml – name: Department of Chemistry
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– name: Centre for Clean Environment and Energy, School of Environment and Science
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  organization: Centre for Advanced 2D Materials and Graphene Research Centre
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Snippet Lithium sulfur (Li–S) battery is considered as one of the most promising energy storage devices, because of its low cost, high energy density, and...
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Title Single-Atom Electrocatalysts for Lithium Sulfur Batteries: Progress, Opportunities, and Challenges
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