Chemistry of Strained Organometallic Rings: Unusual Reactivity of Tin-Bridged [1]Ferrocenophanes with Metal Carbonyls
The reactivity of the stanna[1]ferrocenophane Fe(η-C5H4)2Sn(tBu)2 (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4 fragment into an Sn−Cp bond of 8 was observed on treatment with Fe2(CO)9, forming the ferrostanna[2]ferrocenophane 9 whereas in the case of Co2(CO)8, a hi...
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| Published in | Organometallics Vol. 21; no. 12; pp. 2359 - 2361 |
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| Main Authors | , , , |
| Format | Journal Article |
| Language | English |
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American Chemical Society
10.06.2002
Amer Chemical Soc |
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| Abstract | The reactivity of the stanna[1]ferrocenophane Fe(η-C5H4)2Sn(tBu)2 (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4 fragment into an Sn−Cp bond of 8 was observed on treatment with Fe2(CO)9, forming the ferrostanna[2]ferrocenophane 9 whereas in the case of Co2(CO)8, a highly unusual rearrangement/transfer of CO occurred, forming the ketone-bridged dimer 10. |
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| AbstractList | The reactivity of the stanna[1]ferrocenophane Fe(η-C5H4)2Sn(tBu)2 (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4 fragment into an Sn−Cp bond of 8 was observed on treatment with Fe2(CO)9, forming the ferrostanna[2]ferrocenophane 9 whereas in the case of Co2(CO)8, a highly unusual rearrangement/transfer of CO occurred, forming the ketone-bridged dimer 10. The reactivity of the stanna[1]ferrocenophane Fe(eta-C5H4)(2)Sn(tBu)(2) (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4 fragment into an Sn-Cp bond of 8 was observed on treatment with Fe-2(CO)(9), forming the ferrostanna[2]ferrocenophane 9 whereas in the case Of Co-2(CO)(8), a highly unusual rearrangement/transfer of CO occurred, forming the ketone-bridged dimer 10. |
| Author | Berenbaum, Andrea Lough, Alan J Manners, Ian Jäkle, Frieder |
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| CitedBy_id | crossref_primary_10_1002_anie_200501155 crossref_primary_10_1002_ange_200604409 crossref_primary_10_1002_ange_200454022 crossref_primary_10_1002_chem_200700961 crossref_primary_10_1016_j_ccr_2015_09_008 crossref_primary_10_1021_om3012129 crossref_primary_10_1002_anie_200454022 crossref_primary_10_1002_chem_201100919 crossref_primary_10_1002_zaac_201500557 crossref_primary_10_1002_chem_200700420 crossref_primary_10_1002_ejic_201301144 crossref_primary_10_1021_om400488k crossref_primary_10_1016_j_ica_2004_01_034 crossref_primary_10_1002_ange_200501155 crossref_primary_10_1002_anie_200604409 |
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| Keywords | PHOSPHORUS ROUTE ELEMENTS FERROCENOPHANES TRANSITION-METAL OPENING POLYMERIZATION ROP |
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| Snippet | The reactivity of the stanna[1]ferrocenophane Fe(η-C5H4)2Sn(tBu)2 (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4 fragment into... The reactivity of the stanna[1]ferrocenophane Fe(eta-C5H4)(2)Sn(tBu)(2) (8) toward transition-metal carbonyls was investigated. Insertion of an Fe(CO)4... |
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| SubjectTerms | Chemistry Chemistry, Inorganic & Nuclear Chemistry, Organic Physical Sciences Science & Technology |
| Title | Chemistry of Strained Organometallic Rings: Unusual Reactivity of Tin-Bridged [1]Ferrocenophanes with Metal Carbonyls |
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