Flexible Cobalt-Embedded Carbon Nanosheet/Carbon Nanofiber Composites for Enhanced Electromagnetic Wave Absorption Performance

The rational design of multicomponent materials with tunable microstructures has demonstrated remarkable advantages for attenuating electromagnetic waves (EMWs). Herein, flexible Co-embedded carbon nanosheets/carbon nanofibers (Co@CNSs@CNFs) with three-dimensional structures were prepared by the com...

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Published inACS applied nano materials Vol. 6; no. 7; pp. 5404 - 5413
Main Authors Wen, Bo, Zhou, Ziyi, Wang, Silan, Zhao, Hongyang, Yang, Guorui, Wang, Jiuhong, Niu, Jiaxi, Miao, Yunzi, Zhang, Zhijie, Yan, Wei, Ding, Shujiang
Format Journal Article
LanguageEnglish
Published American Chemical Society 14.04.2023
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Abstract The rational design of multicomponent materials with tunable microstructures has demonstrated remarkable advantages for attenuating electromagnetic waves (EMWs). Herein, flexible Co-embedded carbon nanosheets/carbon nanofibers (Co@CNSs@CNFs) with three-dimensional structures were prepared by the combination of electrospinning and in situ deposition methods, which demonstrate a high specific surface area (62.2 m2 g–1) and rich interfaces between the cobalt nanoparticle and the carbon matrix confirmed by the investigations of scanning electron microscopy (SEM) and transmission electron microscopy (TEM). As a result, the products achieved a broad effective absorption bandwidth of 5.6 GHz and a strong reflection loss of −76.5 dB with a thin thickness of 2.2 mm. It is found that the affluent electromagnetic wave transmission paths and enhanced interfacial polarization loss are the primary reason for the improvement of the EMW absorption performance. This work proposes a tailored way to fabricate the assembled three-dimensional structure and boost EMW absorption through the synergistic effect of multiple polarization loss mechanisms.
AbstractList The rational design of multicomponent materials with tunable microstructures has demonstrated remarkable advantages for attenuating electromagnetic waves (EMWs). Herein, flexible Co-embedded carbon nanosheets/carbon nanofibers (Co@CNSs@CNFs) with three-dimensional structures were prepared by the combination of electrospinning and in situ deposition methods, which demonstrate a high specific surface area (62.2 m2 g–1) and rich interfaces between the cobalt nanoparticle and the carbon matrix confirmed by the investigations of scanning electron microscopy (SEM) and transmission electron microscopy (TEM). As a result, the products achieved a broad effective absorption bandwidth of 5.6 GHz and a strong reflection loss of −76.5 dB with a thin thickness of 2.2 mm. It is found that the affluent electromagnetic wave transmission paths and enhanced interfacial polarization loss are the primary reason for the improvement of the EMW absorption performance. This work proposes a tailored way to fabricate the assembled three-dimensional structure and boost EMW absorption through the synergistic effect of multiple polarization loss mechanisms.
Author Miao, Yunzi
Wang, Silan
Yang, Guorui
Wang, Jiuhong
Yan, Wei
Ding, Shujiang
Niu, Jiaxi
Zhou, Ziyi
Zhao, Hongyang
Wen, Bo
Zhang, Zhijie
AuthorAffiliation Xi’an Key Laboratory of Solid Waste Recycling and Resource Recovery, State Key Laboratory of Multiphase Flow in Power Engineering, Department of Environmental Science and Engineering
Xi’an Jiaotong University
School of Chemistry, Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, “Four Joint Subjects One Union” School-Enterprise Joint Research Center for Power Battery Recycling & Circulation Utilization Technology
School of Mechanical Engineering
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electromagnetic wave absorption performance
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