Ingenious Artificial Leaf Based on Covalent Organic Framework Membranes for Boosting CO2 Photoreduction

• Published in: Journal of the American Chemical Society Vol. 145; no. 17; pp. 9520 - 9529
• Main Authors: Gao, Shuaiqi, Zhang, Qian, Su, Xiaofang, Wu, Xiangkun, Zhang, Xia-Guang, Guo, Yingying, Li, Zhiyong, Wei, Jishi, Wang, Huiyong, Zhang, Suojiang, Wang, Jianji
• Format: Journal Article
• Language: English
• Published: American Chemical Society 03.05.2023
• Subjects: carbon dioxide; leaves; longevity; mass transfer; photocatalysis; photoreduction; photosensitizing agents; photosynthesis; value added

Covalent organic frameworks (COFs) hold the potential in converting CO2 with water into value-added fuels and O2 to save the deteriorating ecological environment. However, reaching high yield and selectivity is a grand challenge under metal-, photosensitizer-, or sacrificial reagent-free conditions....