Breathable and Self-Healing Photothermal Superhydrophobic Coating Featuring Exceptional Liquid Impalement Resistance and Anti-/Deicing Capabilities for Concrete Materials
Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Addition...
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| Published in | ACS applied materials & interfaces Vol. 17; no. 12; pp. 18852 - 18868 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
American Chemical Society
26.03.2025
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| Subjects | |
| Online Access | Get full text |
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| Abstract | Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (W e = 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (−15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications. |
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| AbstractList | Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (
= 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (-15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications. Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (We = 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (-15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications.Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (We = 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (-15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications. Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (W e = 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (−15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications. Ice accumulation and moisture condensation pose significant challenges to the longevity and performance of modern architectural materials. Superhydrophobic anti-icing coatings often suffer mechanical and chemical degradation, particularly in outdoor settings subject to heavy rain or impact. Additionally, most existing coatings are airtight, leading to humidity accumulation and potential substrate deterioration, especially in cement-based materials. To address these challenges, we developed a nonfluorinated, breathable superhydrophobic coating by spraying a PDMS-IPDI-TFB supramolecular network (PIT) mixed with polydopamine nanoparticles (PDA NPs). The optimized superhydrophobic coating (PSC-40) exhibits high breathability, prevents blistering or cracking, and demonstrates exceptional mechanical and chemical durability. Remarkably, it withstands high-speed water jet impacts (W ₑ = 16,000) and retains superhydrophobicity after mechanical and chemical damage. The coating also possesses self-healing capabilities via hydrogen bonds and dynamic covalent bonds, enabling recovery under sunlight, room temperature, or underwater conditions. Its anti-icing performance is evident from a delayed water freezing time (−15 °C) of 1610 s and significantly reduced ice adhesion strength (32.6 kPa). Under sunlight, the coating rapidly melts ice droplets and layers within 138 and 695 s, respectively. This work introduces a robust, breathable superhydrophobic coating with self-healing and anti/deicing capabilities, offering scalable solutions for outdoor, concrete-based architectural applications. |
| Author | Ran, Qianping Zhang, Youfa Dong, Lei Shu, Xin Wu, Yuanlong |
| AuthorAffiliation | State Key Laboratory of Engineering Materials for Major Infrastructure and Jiangsu Key Laboratory of Construction Materials, School of Material Science and Engineering State Key Laboratory of High-Performance Civil Engineering Materials Jiangsu Sobute New Materials Co., Ltd |
| AuthorAffiliation_xml | – name: State Key Laboratory of Engineering Materials for Major Infrastructure and Jiangsu Key Laboratory of Construction Materials, School of Material Science and Engineering – name: State Key Laboratory of High-Performance Civil Engineering Materials – name: Jiangsu Sobute New Materials Co., Ltd |
| Author_xml | – sequence: 1 givenname: Yuanlong surname: Wu fullname: Wu, Yuanlong organization: State Key Laboratory of Engineering Materials for Major Infrastructure and Jiangsu Key Laboratory of Construction Materials, School of Material Science and Engineering – sequence: 2 givenname: Lei orcidid: 0000-0001-7371-6681 surname: Dong fullname: Dong, Lei email: leidong@seu.edu.cn organization: State Key Laboratory of Engineering Materials for Major Infrastructure and Jiangsu Key Laboratory of Construction Materials, School of Material Science and Engineering – sequence: 3 givenname: Xin surname: Shu fullname: Shu, Xin organization: Jiangsu Sobute New Materials Co., Ltd – sequence: 4 givenname: Youfa orcidid: 0000-0003-3225-5502 surname: Zhang fullname: Zhang, Youfa organization: State Key Laboratory of Engineering Materials for Major Infrastructure and Jiangsu Key Laboratory of Construction Materials, School of Material Science and Engineering – sequence: 5 givenname: Qianping orcidid: 0000-0002-7074-7076 surname: Ran fullname: Ran, Qianping email: qpran@cnjsjk.cn organization: Jiangsu Sobute New Materials Co., Ltd |
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| SubjectTerms | adhesion ambient temperature Applications of Polymer, Composite, and Coating Materials chemical degradation durability humidity hydrogen hydrophobicity ice liquids longevity nanoparticles rain solar radiation |
| Title | Breathable and Self-Healing Photothermal Superhydrophobic Coating Featuring Exceptional Liquid Impalement Resistance and Anti-/Deicing Capabilities for Concrete Materials |
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