Visible-Light-Active Photocatalysis - Nanostructured Catalyst Design, Mechanisms, and Applications
A comprehensive and timely overview of this important and hot topic, with special emphasis placed on environmental applications and the potential for solar light harvesting. Following introductory chapters on environmental photocatalysis, water splitting, and applications in synthetic chemistry, fur...
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| Main Author | |
|---|---|
| Format | eBook Book |
| Language | English |
| Published |
Weinheim
John Wiley & Sons
2018
Wiley-VCH John Wiley & Sons, Incorporated |
| Edition | 1 |
| Subjects | |
| Online Access | Get full text |
| ISBN | 3527342931 9783527342938 |
| DOI | 10.1002/9783527808175 |
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| Abstract | A comprehensive and timely overview of this important and hot topic, with special emphasis placed on environmental applications and the potential for solar light harvesting. Following introductory chapters on environmental photocatalysis, water splitting, and applications in synthetic chemistry, further chapters focus on the synthesis and design of photocatalysts, solar energy conversion, and such environmental aspects as the removal of water pollutants, photocatalytic conversion of CO2. Besides metal oxide-based photocatalysts, the authors cover other relevant material classes including carbon-based nanomaterials and novel hybrid materials. Chapters on mechanistic aspects, computational modeling of photocatalysis and Challenges and perspectives of solar reactor design for industrial applications complete this unique survey of the subject. With its in-depth discussions ranging from a comprehensive understanding to the engineering of materials and applied devices, this is an invaluable resource for a range of disciplines. |
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| AbstractList | A comprehensive and timely overview of this important and hot topic, with special emphasis placed on environmental applications and the potential for solar light harvesting. Following introductory chapters on environmental photocatalysis, water splitting, and applications in synthetic chemistry, further chapters focus on the synthesis and design of photocatalysts, solar energy conversion, and such environmental aspects as the removal of water pollutants, photocatalytic conversion of CO2. Besides metal oxide-based photocatalysts, the authors cover other relevant material classes including carbon-based nanomaterials and novel hybrid materials. Chapters on mechanistic aspects, computational modeling of photocatalysis and Challenges and perspectives of solar reactor design for industrial applications complete this unique survey of the subject. With its in-depth discussions ranging from a comprehensive understanding to the engineering of materials and applied devices, this is an invaluable resource for a range of disciplines. This comprehensive overview covers all recent aspects and developments in visible light photocatalysis, with a special emphasis on environmental applications and perspectives on solar light harvesting. |
| Author | Ghosh, Srabanti |
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| Notes | Includes bibliographical references and index |
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| Snippet | A comprehensive and timely overview of this important and hot topic, with special emphasis placed on environmental applications and the potential for solar... This comprehensive overview covers all recent aspects and developments in visible light photocatalysis, with a special emphasis on environmental applications... |
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| SubjectTerms | Catalyseurs Catalysis catalyst aat Catalysts Catalysts fast Chemistry & Chemical Engineering Chemistry, Organic Photocatalyse Photocatalysis Photocatalysis fast Photosynthesis -- Molecular aspects Photosynthesis -- Molecular aspects fast Photosynthèse -- Aspect moléculaire |
| TableOfContents | Title Page
Preface
Table of Contents
1. Research Frontiers in Solar Light Harvesting
2. Recent Advances on Photocatalysis for Water Detoxification and CO2 Reduction
3. Fundamentals of Photocatalytic Water Splitting (Hydrogen and Oxygen Evolution)
4. Photoredox Catalytic Activation of Carbon - Halogen Bonds: C-H Functionalization Reactions under Visible Light
5. Black TiO2: The New-Generation Photocatalyst
6. Effect of Modification of TiO2 with Metal Nanoparticles on its Photocatalytic Properties Studied by Time-Resolved Microwave Conductivity
7. Glassy Photocatalysts: New Trend in Solar Photocatalysis
8. Recent Developments in Heterostructure-Based Catalysts for Water Splitting
9. Conducting Polymers Nanostructures for Solar-Light Harvesting
10. Sensitization of TiO2 by Dyes: A Way to Extend the Range of Photocatalytic Activity of TiO2 to the Visible Region
11. Advances in the Development of Novel Photocatalysts for Detoxification
12. Metal-Free Organic Semiconductors for Visible-Light-Active Photocatalytic Water Splitting
13. Solar Photochemical Splitting of Water
14. Recent Developments on Visible-Light Photoredox Catalysis by Organic Dyes for Organic Synthesis
15. Visible-Light Heterogeneous Catalysts for Photocatalytic CO2 Reduction
16. Band-Gap Engineering of Photocatalysts: Surface Modification versus Doping
17. Roles of the Active Species Generated during Photocatalysis
18. Visible-Light-Active Photocatalysis: Nanostructured Catalyst Design, Mechanisms, and Applications
19. Quantum Dynamics Effects in Photocatalysis
20. An Overview of Solar Photocatalytic Reactor Designs and Their Broader Impact on the Environment
21. Conclusions and Future Work
Index 9.4 Synthesis of Conducting Polymer Nanostructures -- 9.4.1 Hard Templates -- 9.4.2 Soft Templates -- 9.4.3 Template Free -- 9.5 Applications of Conducting Polymer -- 9.5.1 Conducting Polymer Nanostructures for Organic Pollutant Degradation -- 9.5.2 Conducting Polymer Nanostructures for Photocatalytic Water Splitting -- 9.5.3 Conducting Polymer‐Based Heterostructures -- 9.6 Conclusion -- References -- Part III Visible Light Active Photocatalysis for Solar Energy Conversion and Environmental Protection -- Chapter 10 Sensitization of TiO2 by Dyes: A Way to Extend the Range of Photocatalytic Activity of TiO2 to the Visible Region -- 10.1 Introduction -- 10.2 Mechanisms Involved in the Use of Dye‐Modified TiO2 Materials for Transformation of Pollutants and Hydrogen Production under Visible Irradiation -- 10.3 Use of Dye‐Modified TiO2 Materials for Energy Conversion in Dye‐Sensitized Solar Cells -- 10.4 Self‐Sensitized Degradation of Dye Pollutants -- 10.5 Use of Dye‐Modified TiO2 for Visible‐Light‐Assisted Degradation of Colorless Pollutants -- 10.6 Water Splitting and Hydrogen Production using Dye‐Modified TiO2 Photocatalysts under Visible Light -- 10.7 Conclusions -- Acknowledgement -- References -- Chapter 11 Advances in the Development of Novel Photocatalysts for Detoxification -- 11.1 Introduction -- 11.2 Theoretical Studies of Photocatalysis -- 11.2.1 Doping and Surface Modification of TiO2 for Bandgap Engineering -- 11.2.2 Alignment of Valence and Conduction Band Edges with Water Oxidation and Reduction Potentials -- 11.2.3 Electron and Hole Localization -- 11.3 Metal‐Doped Photocatalysts for Detoxification -- 11.3.1 High‐Temperature Stable Anatase TiO2 Photocatalyst -- 11.3.2 Main Group Metal Ions on Anatase Stability and Photocatalytic Activity -- 11.3.3 Effect of Transition Metals on Anatase Stability and Photocatalytic Activity 13.5.3 Multicomponent Heterostructures Chapter 7 Glassy Photocatalysts: New Trend in Solar Photocatalysis -- 7.1 Introduction -- 7.2 Fundamentals of H2S Splitting -- 7.2.1 General -- 7.2.2 Thermodynamics of H2S Splitting -- 7.2.3 Role of Photocatalysts -- 7.3 Designing the Assembly for H2S Splitting -- 7.3.1 Standardization of H2S Splitting Setup -- 7.3.2 Interaction of Photocatalyst and Reagent System -- 7.4 Chalcogenide Photocatalysts -- 7.5 Limitations of Powder Photocatalysts -- 7.6 Glassy Photocatalyst: Innovative Approach -- 7.6.1 Semiconductor-Glass Nanocomposites and Their Advantages -- 7.7 General Methods for Glasses Preparation -- 7.7.1 Glass by Melt‐Quench Technique -- 7.8 Color of the Glass - Bandgap Engineering by Growth of Semiconductors in Glass -- 7.9 CdS-Glass Nanocomposite -- 7.10 Bi2S3-Glass Nanocomposite -- 7.11 Ag3PO4-Glass Nanocomposite -- 7.12 Summary -- Acknowledgments -- References -- Chapter 8 Recent Developments in Heterostructure‐Based Catalysts for Water Splitting -- 8.1 Introduction -- 8.1.1 Band Alignment -- 8.2 Visible‐Light‐Responsive Junctions -- 8.2.1 BiVO4‐Based Junctions -- 8.2.1.1 BiVO4/WO3 -- 8.2.1.2 BiVO4/ZnO -- 8.2.1.3 BiVO4/TiO2 -- 8.2.1.4 BiVO4/Carbon‐Based Materials -- 8.2.2 Fe2O3‐Based Junctions -- 8.2.3 WO3‐Based Junctions -- 8.2.4 C3N4‐Based Junctions -- 8.2.5 Cu2O‐Based Junctions -- 8.3 Visible‐Light‐Driven Photocatalyst/OEC Junctions -- 8.3.1 BiVO4/OEC -- 8.3.2 Fe2O3/OEC -- 8.3.3 WO3/OEC -- 8.4 Observation of Charge Carrier Kinetics in Heterojunction Structure -- 8.4.1 Transient Absorption Spectroscopy -- 8.4.2 Electrochemical Impedance Spectroscopy -- 8.4.3 Surface Photovoltage Spectroscopy -- 8.5 Conclusions -- References -- Chapter 9 Conducting Polymers Nanostructures for Solar‐Light Harvesting -- 9.1 Introduction -- 9.2 Conducting Polymers as Organic Semiconductor -- 9.3 Conducting Polymer‐Based Nanostructured Materials Chapter 4 Photoredox Catalytic Activation of Carbon-Halogen Bonds: C-H Functionalization Reactions under Visible Light -- 4.1 Introduction -- 4.2 Activation of Alkyl Halides -- 4.3 Activation of Aryl Halides -- 4.4 Factors That Determine the Carbon-Halogen Bond Activation of Aryl Halides -- 4.5 Factors That Determine the Yields of the C-H Arylated Products -- 4.6 Achievements and Challenges Ahead -- 4.7 Conclusion -- References -- Part II Design and Developments of Visible Light Active Photocatalysis -- Chapter 5 Black TiO2: The New‐Generation Photocatalyst -- 5.1 Introduction -- 5.2 Designing Black TiO2 Nanostructures -- 5.3 Black TiO2 as Photocatalyst -- 5.4 Conclusions -- References -- Chapter 6 Effect of Modification of TiO2 with Metal Nanoparticles on Its Photocatalytic Properties Studied by Time‐Resolved Microwave Conductivity -- 6.1 Introduction -- 6.2 Deposition of Metal Nanoparticles by Radiolysis and by Photodeposition Method -- 6.3 Electronic Properties Studied Time‐Resolved Microwave Conductivity -- 6.3.1 Surface Modification of Titania with Monometallic Nanoparticles -- 6.3.1.1 Surface Modification of Titania with Pt Clusters -- 6.3.1.2 Surface Modification of TiO2 with Pd Nanoparticles -- 6.3.1.3 Modification of TiO2 with Ag Nanoparticles -- 6.4 Modification of TiO2 with Au Nanoparticles -- 6.5 Modification of TiO2 with Bi Clusters -- 6.6 Surface Modification of TiO2 with Bimetallic Nanoparticles -- 6.6.1 Surface Modification with Au-Cu Nanoparticles -- 6.6.2 Surface Modification with Ag and CuO Nanoparticles -- 6.6.3 Comodification of TiO2 with Ni and Au Nanoparticles for Hydrogen Production -- 6.6.4 TiO2 Modified with NiPd Nanoalloys for Hydrogen Evolution -- 6.7 The Effect of Metal Cluster Deposition Route on Structure and Photocatalytic Activity of Mono‐ and Bimetallic Nanoparticles Supported on TiO2 -- 6.8 Summary -- References Cover -- Title Page -- Copyright -- Contents -- Preface -- Part I Visible‐Light Active Photocatalysis - Research and Technological Advancements -- Chapter 1 Research Frontiers in Solar Light Harvesting -- 1.1 Introduction -- 1.2 Visible‐Light‐Driven Photocatalysis for Environmental Protection -- 1.3 Photocatalysis for Water Splitting -- 1.4 Photocatalysis for Organic Transformations -- 1.5 Mechanistic Studies of Visible‐Light‐Active Photocatalysis -- 1.6 Summary -- References -- Chapter 2 Recent Advances on Photocatalysis for Water Detoxification and CO2 Reduction -- 2.1 Introduction -- 2.2 Photocatalysts for Environmental Remediation and CO2 Reduction -- 2.2.1 Undoped TiO2 -- 2.2.2 Undoped Metal Oxides Different from TiO2 -- 2.2.3 Carbon Modified Metal Oxides as Photocatalysts -- 2.2.4 Doped Metal Oxides -- 2.2.5 Perovskites -- 2.2.6 Metal Chalcogenides -- 2.2.7 Other Catalysts -- 2.3 Photoreactors for Solar Degradation of Organic Pollutants and CO2 Reduction -- 2.3.1 Non Concentrating (Low Concentration or Low Temperature) Systems -- 2.3.2 Medium Concentrating or Medium Temperature Systems -- 2.3.3 High Concentrating or High‐Temperature Systems -- 2.3.4 Parameters of a Solar Reactor -- 2.4 Conclusion -- Acknowledgment -- References -- Chapter 3 Fundamentals of Photocatalytic Water Splitting (Hydrogen and Oxygen Evolution) -- 3.1 Introduction -- 3.2 Strategy for Development of Photocatalyst Systems for Water Splitting -- 3.3 Electrochemistry of Semiconductors at the Electrolyte Interface -- 3.4 Effect of Light at the Semiconductor-Electrolyte Interface -- 3.5 Conversion and Storage of Sunlight -- 3.6 Electrolysis and Photoelectrolysis -- 3.7 Development of Photocatalysts for Solar‐Driven Water Splitting -- 3.8 Approaches to Develop Visible‐Light‐Absorbing Metal Oxides -- 3.9 Conclusions -- References 11.3.4 Effect of Rare Earth Metal Ions on Anatase Stability and Photocatalytic Activity -- 11.4 Graphene‐TiO2 Composites for Detoxification -- 11.5 Commercial Applications of Photocatalysis in Environmental Detoxification -- 11.5.1 Self‐Cleaning Materials -- 11.5.2 Bactericidal -- 11.5.3 Wastewater Detoxification -- 11.6 Conclusions -- References -- Chapter 12 Metal‐Free Organic Semiconductors for Visible‐Light‐Active Photocatalytic Water Splitting -- 12.1 Introduction -- 12.2 Organic Semiconductors for Photocatalytic Water Splitting and Emergence of Graphitic Carbon Nitrides -- 12.3 Graphitic Carbon Nitrides for Photocatalytic Water Splitting -- 12.3.1 Precursor‐Derived g‐CN -- 12.3.2 Nanoporous g‐CN by Templating Methods -- 12.3.2.1 Hard Templating -- 12.3.2.2 Soft Templating -- 12.3.2.3 Template‐Free -- 12.3.3 Heteroatom Doping -- 12.3.3.1 Metal Doping -- 12.3.3.2 Nonmetal Doping -- 12.3.4 Metal Oxides/g‐CN Nanocomposites -- 12.3.5 Graphene and CNT‐Based g‐CN Nanocomposites -- 12.3.6 Structural Modification with Organic Groups -- 12.3.7 Crystalline Carbon Nitrides -- 12.3.8 Overall Water Splitting and Large‐Scale Hydrogen Production Using Carbon Nitrides -- 12.4 Novel Materials -- 12.4.1 Triazine and Heptazine‐Based Organic Polymers -- 12.4.2 Covalent Organic Frameworks (COFs) and Beyond -- 12.5 Conclusions and Perspectives -- References -- Chapter 13 Solar Photochemical Splitting of Water -- 13.1 Introduction -- 13.2 Photocatalytic Water Splitting -- 13.2.1 Fundamentals of Water Splitting -- 13.2.2 Light‐Harvesting Units -- 13.2.3 Photocatalytic Activity -- 13.2.4 Effect of Size of Nanostructures -- 13.3 Overall Water Splitting -- 13.3.1 One‐Step Photocatalytic Process -- 13.3.2 Two‐Step (Z‐Scheme) Photocatalytic Process -- 13.4 Oxidation of Water -- 13.5 Reduction of Water -- 13.5.1 C3N4 and Related Materials -- 13.5.2 Semiconductors |
| Title | Visible-Light-Active Photocatalysis - Nanostructured Catalyst Design, Mechanisms, and Applications |
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