Spatially Patterned Architectures to Modulate CO2 Reduction Cascade Catalysis Kinetics

• Published in: ACS catalysis Vol. 15; no. 7; pp. 5894 - 5905
• Main Authors: García-Batlle, Marisé, Fernandez, Pablo, Sheehan, Colton J., He, Shi, Mallouk, Thomas E., Parsons, Gregory N., Cahoon, James F., Lopez, Rene
• Format: Journal Article
• Language: English
• Published: American Chemical Society 04.04.2025
• Subjects: spatial rearrangement; cascade catalysis; modeling; CO2 reduction; COMSOL; geometrical parametrization
• ISSN: 2155-5435; 2155-5435
• DOI: 10.1021/acscatal.5c01176

Electrochemical CO2 reduction using renewable sources of electrical energy holds promise for converting CO2 into fuels and chemicals. The complex interactions among chemical/electrochemical reactions and mass transport make it difficult to analyze the effect of an individual process on electrode per...